Physicochemical Characterization of Microplastics in Refillable Water Gallon Containers
##doi.readerDisplayName##:
https://doi.org/10.65166/jnrrwf32关键词:
microplastics, refillable water containers, drinking water quality, FTIR spectroscopy, polyamide, environmental health摘要
Microplastic contamination in drinking water has become an emerging environmental health concern, particularly in communities that rely on refillable water gallon containers for household consumption. This study aimed to determine the presence, physical characteristics, and chemical composition of microplastics in drinking water collected from refillable water gallon containers used by selected households in Barangay 641, San Miguel, Manila. A descriptive-quantitative research design was employed. Twenty 250-mL water samples were collected and subjected to vacuum filtration using a 0.45 µm membrane filter. The retained particles were examined through USB digital microscopy and the Hot Needle Test to screen, classify, count, and measure suspected microplastics. Representative particles were further analyzed using Fourier Transform Infrared spectroscopy to identify probable polymer composition. Results showed that 12 out of 20 samples, or 60%, tested positive for microplastics. A total of 32 microplastic particles were detected, with an average of 1.6 particles per 250-mL sample. The particles were classified as fibers and microfibers, each accounting for 50% of the detected particles. Fibers ranged from 1.01 to 3.22 mm, while microfibers ranged from 0.27 to 0.95 mm. FTIR analysis identified the representative particles as probable polyamide based on characteristic absorption peaks. The findings provide baseline evidence of microplastic occurrence in refillable water gallon samples and support the need for improved monitoring, handling practices, and consumer safety assessment in refillable drinking-water systems.
##plugins.themes.default.displayStats.downloads##
参考
Adib, D., Mafigholami, R., & Tabeshkia, H. (2021). Identification of microplastics in conventional drinking water treatment plants in Tehran, Iran. Journal of Environmental Health Science and Engineering, 19(2), 1817–1826. https://doi.org/10.1007/s40201-021-00737-3
Altunışık, A. (2023). Microplastic pollution and human risk assessment in Turkish bottled natural and mineral waters. Environmental Science and Pollution Research, 30(14), 39815–39825. https://doi.org/10.1007/s11356-022-25054-6
Arcadio, C. G. L. A., Navarro, C. K. P., Similatan, K. M., Inocente, S. A. T., Ancla, S. M. B., Banda, M. H. T., Capangpangan, R. Y., Torres, A. G., & Bacosa, H. P. (2022). Microplastics in surface water of Laguna de Bay: First documented evidence on the largest lake in the Philippines. Environmental Science and Pollution Research, 30(11), 30524–30533. https://doi.org/10.1007/s11356-022-24261-5
Atento, A. G., & Atento, R. G. (2025). A case study of Mercury Drug Corporation: Strategic adaptation to universal healthcare and digital disruption in the Philippines. International Journal of Health & Business Analytics, 1(1). https://doi.org/10.65166/zhw7dd39
Atento, R. G. (2025). Exploring e-learning for sustainable development: Integrating SDGs in management education at Philippine higher education institutions. International Journal of Health & Business Analytics, 1(1). https://doi.org/10.65166/2qcjx561
Atento, R. G., Quinto, L., Espelita, C. A. M., & Castaneda, C. (2025). Integrating business and health analytics: A conceptual framework for dual outcomes in healthcare. International Journal of Health & Business Analytics, 1(1). https://doi.org/10.65166/04pdc866
Blackburn, K., & Green, D. (2021). The potential effects of microplastics on human health: What is known and what is unknown. Ambio, 51(3), 518–530. https://doi.org/10.1007/s13280-021-01589-9
Borenstein, S. (2024, January 8). Scientists find about a quarter million invisible microplastic particles in a liter of bottled water. PBS News. https://www.pbs.org/newshour/science/scientists-find-about-a-quarter-million-invisible-microplastic-particles-in-a-liter-of-bottled-water
Cao, N., Vo, D. T., Pham, M., Nguyen, V., Nguyen, T., Le, L., Mukhtar, H., Nguyen, H., Visvanathan, C., & Bui, X. (2024). Microplastics contamination in water supply system and treatment processes. Science of the Total Environment, 926, 171793. https://doi.org/10.1016/j.scitotenv.2024.171793
Catilogo, M. I. U. (2023, March 23). PHL access to drinking water improves; 54% source from commercial refilling stations. BusinessWorld Online. https://www.bworldonline.com/the-nation/2023/03/23/512553/phl-access-to-drinking-water-improves-54-source-from-commercial-refilling-stations/
Chandra, S., & Walsh, K. B. (2024). Microplastics in water: Occurrence, fate and removal. Journal of Contaminant Hydrology, 264, 104360. https://doi.org/10.1016/j.jconhyd.2024.104360
Culpepper, J. (2023, October 3). What’s in your water bottle? Concerns about microplastics in caps. Environmental Working Group. https://www.ewg.org/news-insights/news/2023/10/whats-your-water-bottle-concerns-about-microplastics-caps
Department of Health. (2017, June 23). Administrative Order No. 2017-0010: Philippine National Standards for Drinking Water of 2017. https://www.fda.gov.ph/wp-content/uploads/2021/08/Administrative-Order-No.-2017-0010.pdf
Espiritu, E. Q., Pauco, J. L. R., Bareo, R. S., Palaypayon, G. B., Capistrano, H. A. M., Jabar, S. R., Coronel, A. S. O., Rodolfo, R. S., & Enriquez, E. P. (2024). Microplastics contamination in selected staple consumer food products. Journal of Food Science and Technology, 61(11), 2082–2092. https://doi.org/10.1007/s13197-024-05978-2
Gambino, I., Bagordo, F., Grassi, T., Panico, A., & De Donno, A. (2022). Occurrence of microplastics in tap and bottled water: Current knowledge. International Journal of Environmental Research and Public Health, 19(9), 5283. https://doi.org/10.3390/ijerph19095283
Hee, Y. Y., Weston, K., & Suratman, S. (2022). The effect of storage conditions and washing on microplastic release from food and drink containers. Food Packaging and Shelf Life, 32, 100826. https://doi.org/10.1016/j.fpsl.2022.100826
Hu, J., Duan, Y., Zhong, H., Lin, Q., Zhang, T., Zhao, C., Chen, S., Dong, B., Li, D., Wang, J., Mo, M., Chen, J., & Zheng, J. (2022). Analysis of microplastics released from plastic take-out food containers based on thermal properties and morphology study. Food Additives & Contaminants: Part A, 40(2), 305–318. https://doi.org/10.1080/19440049.2022.2157894
Kelishadi, R., Beni, A. A., Ebrahimpour, K., & Heidari-Beni, M. (2024). Determination of microplastic release from disposable plastic containers in Isfahan. Chinese Journal of Analytical Chemistry, 100448. https://doi.org/10.1016/j.cjac.2024.100448
Kumar, R., Manna, C., Padha, S., Verma, A., Sharma, P., Dhar, A., Ghosh, A., & Bhattacharya, P. (2022). Micro(nano)plastics pollution and human health: How plastics can induce carcinogenesis to humans? Chemosphere, 298, 134267. https://doi.org/10.1016/j.chemosphere.2022.134267
Li, Y., Tao, L., Wang, Q., Wang, F., Li, G., & Song, M. (2023). Potential health impact of microplastics: A review of environmental distribution, human exposure, and toxic effects. Environment & Health, 1(4), 249–257. https://doi.org/10.1021/envhealth.3c00052
Menon, V., Sharma, S., Gupta, S., Ghosal, A., Nadda, A. K., Jose, R., Sharma, P., Kumar, S., Singh, P., & Raizada, P. (2023). Prevalence and implications of microplastics in potable water system: An update. Chemosphere, 317, 137848. https://doi.org/10.1016/j.chemosphere.2023.137848
Nacino, G. E., & Basit, S. A. (2025). Microplastics, bacterial isolates, and antimicrobial resistance profiles in Decapterus macrosoma from Cavite, Philippines. International Journal of Health & Business Analytics, 1(2). https://doi.org/10.65166/bevs3330
National Oceanic and Atmospheric Administration. (2024, June 16). What are microplastics? https://oceanservice.noaa.gov/facts/microplastics.html
Natsir, M. F., Amaludin, A., Rasyid, B., & Arsin, A. A. (2025). Microplastic contamination in refilled drinking water: The impact of gallon washing frequency. Journal of Ecological Engineering, 26(12), 221–228. https://doi.org/10.12911/22998993/208486
O’Brien, S., Rauert, C., Ribeiro, F., Okoffo, E. D., Burrows, S. D., O’Brien, J. W., Wang, X., Wright, S. L., & Thomas, K. V. (2023). There’s something in the air: A review of sources, prevalence and behaviour of microplastics in the atmosphere. Science of the Total Environment, 874, 162193. https://doi.org/10.1016/j.scitotenv.2023.162193
Osorio, E. D., Tanchuling, M. A. N., & Diola, M. B. L. D. (2021). Microplastics occurrence in surface waters and sediments in five river mouths of Manila Bay. Frontiers in Environmental Science, 9, Article 719274. https://doi.org/10.3389/fenvs.2021.719274
Plastic Pollution Coalition. (2024, March 4). Study finds hundreds of thousands of plastic particles in bottled water. https://www.plasticpollutioncoalition.org/blog/2024/1/10/study-finds-hundreds-of-thousands-of-plastic-particles-in-bottled-water
Polychronopoulos, N. D., & Vlachopoulos, J. (2023). On the origin of microplastics in bottled water. AIP Conference Proceedings, 2884, 180001. https://doi.org/10.1063/5.0168577
Romarate, R. A., Ancla, S. M. B., Patilan, D. M. M., Inocente, S. A. T., Pacilan, C. J. M., Sinco, A. L., Guihawan, J. Q., Capangpangan, R. Y., Lubguban, A. A., & Bacosa, H. P. (2023). Breathing plastics in Metro Manila, Philippines: Presence of suspended atmospheric microplastics in ambient air. Environmental Science and Pollution Research, 30(18), 53662–53673. https://doi.org/10.1007/s11356-023-26117-y
Rosariawari, F., Abdulloh, M. N., & Fitriani, N. (2021). Identification of microplastic content in refilled drinking water in the district of Gunung Anyar Surabaya, Indonesia. Pollution Research, 40(1). https://www.envirobiotechjournals.com/PR/v40i12021/Poll%20Res-28.pdf
Sajorne, R. E., Cayabo, G. D. B., Gajardo, L. J. A., Mabuhay-Omar, J. A., Creencia, L. A., & Bacosa, H. P. (2022). Disentangling microplastic pollution on beach sand of Puerto Princesa, Palawan Island, Philippines: Abundance and characteristics. Sustainability, 14(22), 15303. https://doi.org/10.3390/su142215303
Schymanski, D., Oßmann, B. E., Benismail, N., Boukerma, K., Dallmann, G., Von Der Esch, E., Fischer, D., Fischer, F., Gilliland, D., Glas, K., Hofmann T., Käppler, A., Lacorte, S., Marco, J., Rakwe, M. E., Weisser, J., Witzig, C., Zumbülte, N., & Ivleva, N. P. (2021). Analysis of microplastics in drinking water and other clean water samples with micro-Raman and micro-infrared spectroscopy: Minimum requirements and best practice guidelines. Analytical and Bioanalytical Chemistry, 413(24), 5969–5994. https://doi.org/10.1007/s00216-021-03498-y
Singh, S., Trushna, T., Kalyanasundaram, M., Tamhankar, A. J., & Diwan, V. (2022). Microplastics in drinking water: A macro issue. Water Science & Technology: Water Supply, 22(5), 5650–5674. https://doi.org/10.2166/ws.2022.189
Sumam, S. B., Gautam, S., & Arulraj, P. (2025). Understanding microplastic pollution in groundwater: Pathways, health implications and solutions. Water Environment Research, 97(7). https://doi.org/10.1002/wer.70132
Sun, A., & Wang, W. (2023). Human exposure to microplastics and its associated health risks. Environment & Health, 1(3), 139–149. https://doi.org/10.1021/envhealth.3c00053
Temporada, K., Quinto, L., Tarraya, D. A., Sison, F. C., Marfil, J. F., Ramirez, C., & Ng, W. J. (2025). Awareness and preventive practices on leptospirosis in flood-prone communities of Marikina City, Philippines. International Journal of Health & Business Analytics, 1(1). https://doi.org/10.65166/x71zvx65
Tirkey, A., & Upadhyay, L. S. B. (2021). Microplastics: An overview on separation, identification and characterization of microplastics. Marine Pollution Bulletin, 170, 112604. https://doi.org/10.1016/j.marpolbul.2021.112604
Velmurugan, P., Vijayaprabhakaran, N. K., & Devika, P. (2023). Baseline study on identification, characterization, distribution and abundance of microplastics in surface water from Ennore to Kovalam along the east coast of India. Physics and Chemistry of the Earth, Parts A/B/C, 130, 103391. https://doi.org/10.1016/j.pce.2023.103391
Weber, F., Kerpen, J., Wolff, S., Langer, R., & Eschweiler, V. (2021). Investigation of microplastics contamination in drinking water of a German city. Science of the Total Environment, 755, 143421. https://doi.org/10.1016/j.scitotenv.2020.143421
Weisser, J., Beer, I., Hufnagl, B., Hofmann, T., Lohninger, H., Ivleva, N. P., & Glas, K. (2021). From the well to the bottle: Identifying sources of microplastics in mineral water. Water, 13(6), 841. https://doi.org/10.3390/w13060841
Wong, N., Chai, C., Bamgbade, J., Ma, G., & Hii, G. (2021). Detection of microplastics in bottled water. Materials Science Forum, 1030, 169–176. https://doi.org/10.4028/www.scientific.net/MSF.1030.169
Yang, Q., Peng, Y., Wu, X., Cao, X., Zhang, P., Liang, Z., Zhang, J., Zhang, Y., Gao, P., Fu, Y., Liu, P., Cao, Z., & Ding, T. (2025). Microplastics in human skeletal tissues: Presence, distribution and health implications. Environment International, 196, 109316. https://doi.org/10.1016/j.envint.2025.109316
Ylagan, H. M., Aguirre, K. A. G. C., Briones, L. A., Briones, P. N. P., Canapi, C. V. T., Corpuz, K. M. R., Esmelo, A. J. M., Ganacial, V. J. M., Gasid, K. M. M., Ledesma, A. F. P., Marasigan, K. V. O., Miraples, M. B., Santos, E. G. D., Valdez, J. F. L., & Quinto, L. F. (2025). Post-rehabilitation heavy metal contamination analysis of kangkong (Ipomoea aquatica) cultivated in the Pasig River Waterway, Manggahan Floodway. International Journal of Health & Business Analytics, 1(2). https://doi.org/10.65166/xf4mm102
Ylagan, H., Reyes, J. B., Rakiin, A. M., Atria, A., Paredes, J. B., Margarett, A., Angela, F., Decepeda, D. V., Janine, T., Belviz, J. M., Baro, A. M., Briz, P. J., Quinto, L., Jean, H., & Sesma, G. (2026). Microplastic contamination and gram-negative bacterial profiles in Sardinella fimbriata collected from Manila Bay. International Journal of Health & Business Analytics, 2(1). https://doi.org/10.65166/zt30xk47
Zhao, B., Rehati, P., Yang, Z., Cai, Z., Guo, C., & Li, Y. (2023). The potential toxicity of microplastics on human health. Science of the Total Environment, 912, 168946. https://doi.org/10.1016/j.scitotenv.2023.168946
##submission.downloads##
已出版
##submission.license##
##submission.copyrightStatement##
##submission.license.cc.by-nc-sa4.footer##This work is licensed under a Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International License.
Authors retain copyright of their articles but grant the International Journal of Health & Business Analytics (IJHBA) the right of first publication.